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Chemoselective Minisci Alkylation in Aqueous Medium: A General Strategy for Functionalization of Complex N-Heteroarenes and Biomolecules
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC04621A, PaperQi-Long Hu, Jun-Jie Deng, Jia Ye, Jian Li, Albert S. C. Chan, Hang Su, Xiao-Feng Xiong
Efficiently constructing highly functionalized N-heteroarenes under mild reaction conditions is one of the most important approaches to facilitate the discovery of bioactive molecules. In this context, boronic ester derivatives as...
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DOI: 10.1039/D5GC04621A, PaperQi-Long Hu, Jun-Jie Deng, Jia Ye, Jian Li, Albert S. C. Chan, Hang Su, Xiao-Feng Xiong
Efficiently constructing highly functionalized N-heteroarenes under mild reaction conditions is one of the most important approaches to facilitate the discovery of bioactive molecules. In this context, boronic ester derivatives as...
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Expanding and recycling a water-resistant bioderived rigid foam using CO2-responsive amines and carbonated water
DOI: 10.1039/D4GC06165A, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Daniel Barker, Michael F. Cunningham, Guojun Liu, Philip G. JessopBy combining renewable resources with CO2-responsive functionalities, a sustainable foam packaging material was developed. This bioderived foam can be recycled by dissolving it into carbonated water and expanding it into a new foam product.
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From lignin to market: a technical and economic perspective of reductive depolymerization approaches
DOI: 10.1039/D5GC02316E, Critical Review
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Brent Daelemans, Balaji Sridharan, Paul Jusner, Agneev Mukherjee, Jiazhao Chen, Jacob K. Kenny, Miet Van Dael, Karolien Vanbroekhoven, Peter J. Deuss, Michael L. Stone, Elias FeghaliThe industrial potential of pilot-scale reductive depolymerization approaches is critically assessed from a technical, techno-economic, and application point of view.
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All-climate all-solid-state batteries enabled by high-entropy amorphous oxyhalide solid electrolytes
DOI: 10.1039/D5GC03551A, PaperShufeng Song, Wei Xue, Yumei Wang, Zhongting Wang, Yanming Cui, Zhixu Long, Hongyang Shan, Ning Hu, Jingfeng Wang, Fusheng Pan
A high-entropy mixed-ion strategy overcomes ASSBs’ temperature limits. The engineered high-entropy amorphous oxyhalide achieves high ionic conductivity (7.1 mS cm−1) and enhanced electrochemical stability, enabling all-climate ASSBs.
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A bifunctional recyclable gemini surfactant catalyst for oxidative nitroso Diels-Alder reactions in water
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03912F, PaperLongxia Jia, Hongling Liu, Weiwei Shi, Yingru Xu, Ruihan Sun, Jia Zuo, Bin Wang, Jianjian Huang, Fangrui Zhong, Dangui Wang
A novel bifunctional cationic gemini iodide catalyst was designed for oxidative nitroso Diels-Alder reactions in aqueous media. This surfactant-type catalyst spontaneously self-assembles into micellar nanoreactors in water, facilitating hetero-Diels–Alder reactions...
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DOI: 10.1039/D5GC03912F, PaperLongxia Jia, Hongling Liu, Weiwei Shi, Yingru Xu, Ruihan Sun, Jia Zuo, Bin Wang, Jianjian Huang, Fangrui Zhong, Dangui Wang
A novel bifunctional cationic gemini iodide catalyst was designed for oxidative nitroso Diels-Alder reactions in aqueous media. This surfactant-type catalyst spontaneously self-assembles into micellar nanoreactors in water, facilitating hetero-Diels–Alder reactions...
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Revealing the roles of light and heat for enhanced interfacial charge transfer in photocatalytic conversion of methanol to formaldehyde coupled with hydrogen evolution
DOI: 10.1039/D5GC03911H, PaperHoukui Xiang, Wanqi Liu, Zhaokai Zeng, Jingxian Chen, Beile Lin, Guoliang Zhang, Xuhui Wei, Songbo Zhou, Tongqiang Xiong, Pengfei Li, Libing Qian
Photothermal catalytic methanol (CH3OH) dehydrogenation is a sustainable pathway for the co-production of hydrogen (H2) and formaldehyde (HCHO) under mild reaction conditions.
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Synergistic recycling of polycarbonate: efficient BPA recovery integrated with CO2 utilization to produce valuable chemicals
DOI: 10.1039/D5GC02387D, PaperYue Bai, Minghao Zhang, Siming Zhu, Zhuo Wang, Yu Liu, Jianxiu Hao, Huacong Zhou, Qingqing Mei
This work introduces a synergistic strategy that simultaneously converts PC and its hydrolysis by-product CO2 into high-value products (BPA and PDO), achieving full carbon utilization with no CO2 emissions.
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Photocatalytic transformation of aliphatic heterocycles and electron-poor alkenes into functionalized heteroarenes
DOI: 10.1039/D5GC04418A, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Lorenzo Di Terlizzi, Davide Ravelli, Burkhard KönigThe merger of decatungstate photocatalysis and cobaloxime catalysis enabled the preparation of functionalized heteroarenes via a hydroalkylation/aromatization sequence starting from largely available aliphatic heterocycles and electron-poor olefins.
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Scalable glycolysis-based depolymerization of polyurethane foam waste enabled by ionic liquids
DOI: 10.1039/D5GC03643G, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Francisco Velasco, Rocio Villa, Nicolas Alonso, Rebeca Salas, Jairton Dupont, Eduardo Garcia-Verdugo, Pedro LozanoA sustainable and scalable strategy for the glycolytic depolymerization of polyurethane foam (PUF) waste, based on the ionic liquid technology under mild conditions, provides a suitable starting material for re-synthesis of new flexible PUF.
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Interface engineering via in situ constructed zincophilic gradient interphases for high-performance zinc-ion batteries in wide temperature ranges
DOI: 10.1039/D5GC03908H, PaperYi-Yang Bi, Song-Lin Tian, Yang Yu, Yu Zhang, Lian-Shan Sun, Jian Li, Wan-Qiang Liu, Kai Li, Gang Huang
With the steadily rising demand for energy storage devices, there is an increasing need for high-performance batteries.
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Catalytic vapour phase hydrodehalogenation of 1,8-dichlorooctane over Pd@MIL-101(Cr)-NH2: a step forward in MOF-based technologies
DOI: 10.1039/D5GC04671H, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Raúl M. Guerrero, Ignacio D. Lemir, Carlos Fernández-Ruiz, Sergio Carrasco, Patricia Horcajada, David P. Serrano, Yolanda Pérez, Patricia PizarroCatalytic hydrodehalogenation (HDH) represents a promising strategy to remove halogens (Cl and Br) in pyrolysis oils derived from halogenated plastic waste.
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A comprehensive review on hydrothermal humic acids: synthesis, characterization, applications, and perspectives
DOI: 10.1039/D5GC03926F, Tutorial ReviewHu Xu, Yangyang Li, Yexuan He, Xin Sheng, Zhiwei Zhao, Li Li
The synthesis and application of hydrothermal humic acids represent a carbon-negative pathway, analogous to the significance of basketball as a vital form of exercise.
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Intensifying hydrogen spillover over silicotungstic acid decorated carbon black-supported Ru by green plasma preparation for boosting the electrocatalytic hydrogen evolution reaction
DOI: 10.1039/D5GC03845F, PaperYunzhe Ma, Hong Li, Fei Gao, Yue Hua, Xiuling Zhang, Jingsen Zhang, Lanbo Di
Green plasma preparation intensified hydrogen spillover over silicotungstic acid decorated carbon black-supported Ru for boosting HER performance.
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An unconventional photochemical amide synthesis from excited-state nitroarenes
DOI: 10.1039/D5GC03649F, PaperZengping Wang, Xiaofang Zhai, Pengtao Bai, Li Fang, Shaojun Zheng, Jiajia Zhao, Fu Yang, Chen Xu, Heng Song
Based on the bifunctional nature of photoexcited nitroarenes, a novel photochemical approach for amide synthesis was developed.
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Mechanochemical ball milling as an emerging tool in chemical recycling and upcycling of waste polymers
DOI: 10.1039/D5GC03507D, Critical Review
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Anamarija Briš, Davor Margetić, Vjekoslav ŠtrukilA comprehensive review of mechanochemical recycling and upcycling of waste polymers by ball milling is critically assessed, highlighting its efficiency and potential for the depolymerization or degradation of waste plastics.
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2-Methyl-2-(pyridin-2-yl)malononitrile: a site-selective cyano transfer reagent for photocatalytic cyanation reactions
DOI: 10.1039/D5GC03425F, PaperXiang-Chuang Tan, Lei Yan, Hao-Ni Qin, Peng-Fei Xu
Herein, we report the development of a carbon-bound radical cyanating reagent, 2-methyl-2-(pyridin-2-yl)malononitrile (MPYMN), which enables metal-free photocatalytic cyanation with high reactivity and site selectivity.
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Interfacial engineering-triggered electronic regulation of Re and CoP hollow multi-shelled structure toward high-activity electrochemical water splitting
DOI: 10.1039/D5GC03290C, PaperGuangyao Zhou, Mingxin Pang, Jing Li, Bin He, Zhijuan Li, Yawen Tang
Cooperation between interfacial engineering and a hollow multi-shelled structure boosts the water electrolysis performance of Re/CoP.
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Short and sustainable synthesis of the anticancer agent tepotinib
DOI: 10.1039/D5GC04089B, CommunicationEduam O. Boeira, Angélica V. Moro, Bruce H. Lipshutz
Synthesis of the anticancer drug tepotinib was achieved in only 5 steps (3 steps in the longest linear sequence), with an overall yield of 75%.
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Eco-friendly synthesis of imine-based COFs for efficient photocatalytic H2O2 production
DOI: 10.1039/D5GC03415A, PaperYayang Wang, Ting Xu, Zhongxing Zhang, Yaowen Wang, Jiming Huang, Mi Tang, Zhengbang Wang
Imine-based COFs, synthesized via eco-friendly methods, enable efficient visible-light-driven H2O2 production with excellent photocatalytic performance.
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Ionic liquid-mediated solid–liquid extraction and separation processes for essential oils: modern trends
DOI: 10.1039/D5GC01303H, PerspectivePankaj Kumar, Sonali Khanal, Isha Soni, Pooja Shandilya, Manish Kumar, Dinesh Kumar, Tejwant Singh Kang, Vinay Chauhan
Ionic liquids (ILs) have proven to be a potential medium for the extraction and separation of essential oils (EOs) from the most varied sources.
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