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Performance of composite oxygen carriers for plasma-assisted nitrogen fixation and ammonia synthesis
DOI: 10.1039/D5GC06222E, PaperBaiqiang Zhang, Yongqi Liang, Jia Wang, Xi Chen, Anqi Li, Yuyang Zhang, Yuhui Chen, Shiquan Zhu, Nobusuke Kobayashi, Bo Wu
High oxygen vacancy (Ov)-rich nitrogen carriers are developed via the synergy between plasma and oxygen carriers, significantly enhancing NH3 yield.
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Nitrogen source-regulated biomass-based COF@CNF aerogel: achieving efficient photothermal–photocatalytic synergy
DOI: 10.1039/D6GC01211F, PaperRanran Ji, Yaning Xu, Menglu Yang, Chengxu Zhou, Tiantian Wu, Yujie Zhao, Qing Huang, Dan Tian
A COF@CNF evaporator integrating aligned CNF microchannels and nitrogen-engineered COFs enables simultaneous efficient solar evaporation and photocatalytic H2O2 production.
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Radical-driven upcycling of spent graphite into defect-controllable nitrogen-doped graphene for sustainable energy storage
DOI: 10.1039/D6GC01392A, PaperXiangfei Zeng, Yunhui Han, Huimin Yang, Hao Li, Anlong Han, Qian Liang, Ling Hu, Rong Wang, Mengjun Chen
Unveiling a radical-driven wedge-cleavage mechanism in suspension electrolysis for the green upcycling of spent battery graphite. This yields high-value N-doped graphene tailored for efficient OER and supercapacitor applications.
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Ionic liquids for sustainable lignin biorefinery: from dissolution mechanisms to electrocatalytic upgrading
DOI: 10.1039/D6GC01240J, Tutorial ReviewZiqi Zhai, Yumiao Lu, Wei-Lu Ding, Yuxuan Guo, Songsong Chen, Hongyan He, Suojiang Zhang
Ionic liquids integrate dissolution and electrocatalysis to overcome lignin recalcitrance, enabling lignin valorization.
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Low-voltage suspension electrolysis enables redox-coupled synergistic leaching for closed-loop recycling of mixed NCM-LFP cathodes
DOI: 10.1039/D6GC01668E, PaperKenan Zhong, Fucheng Wang, Wenke Liu, Zhuo Ye, Xueyang Hou, Kai Yang, Zhao Fang
Low-voltage suspension electrolysis enables reductant-free synergistic leaching of mixed NCM/LFP cathodes via Fe-mediated redox coupling, achieving >98% metal recovery and enabling closed-loop regeneration of battery materials with low energy input.
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Electroreductive divergent hydrolysis and hydrogenation of 2-oxazolidinones
DOI: 10.1039/D6GC01195K, PaperZe-Zhao Huang, Wen-Xi Duan, Fan Li, Yan-Zhao Wang, Jin-Yu He, Cuiju Zhu
Electroreductive divergent hydrolysis and hydrogenation of 2-oxazolidinones for accessing various chiral amino alcohols and amines.
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Scalable and sustainable mechanochemical deracemisation by resonant acoustic mixing
DOI: 10.1039/D5GC06927K, PaperGuillaume Wery, Job Gieling, Zoer El Kaderi, Leeroy Hendrickx, Thomas Wiegand, Carsten Bolm, Tom Leyssens, Daniel M. Baier
Resonant Acoustic Mixing (RAM) presents a scalable, solvent-minimised method for deracemisation, achieving up to 91% enantiomeric enrichment. This approach offers a faster, waste-reducing, and scalable pathway for large-scale deracemisation.
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Two-second surface-confined reconstruction of cellulose paper via a recyclable molten salt hydrate for water-resistant bioplastics
DOI: 10.1039/D6GC01239F, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Ping Wang, Zhonglei Huang, Meiyan Wu, Safoora Mirmohamadsadeghi, Chao Liu, Guang Yu, Haishun Du, Jing Shen, Bin LiTwo-second surface-confined reconstruction upgrades cellulose paper into high-strength, water-resistant bioplastics using recyclable LiBr·3H2O.
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Polymers in ionic liquids and ionic liquids in polymers: critical factors for compatibility and materialization
DOI: 10.1039/D6GC01648K, PerspectiveMasayoshi Watanabe
The compatibility of polymers in ionic liquids (ILs) is governed by the competition between solute–IL and cation–anion interactions. This enables the development of novel IL/polymer materials.
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Improvement of the operational stability and durability of proton exchange membrane fuel cells by using a novel lignin-containing nanocellulose fiber modified carbon fiber paper
DOI: 10.1039/D6GC00753H, PaperRuyin Ma, Yunfei Zhang, Jinghang Zhu, Daliang Guo, Jianbin Chen, Linxin Zhong, Chengliang Duan, Yinchao Xu, Jing Li, Huifang Zhao, Lizheng Sha
Biomass-derived lignin-cellulose nanofiber reinforced carbon paper is used for PEMFCs. The optimized sample demonstrated excellent durability after 4000 cycles, while balancing strength, conductivity and cost.
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Photocatalytic CO2-promoted divergent C(sp3)–H carboxylation of benzyl alcohols
DOI: 10.1039/D6GC02235A, PaperWenlong Shan, Zeyu Zhang, Jiayuan Li, Chanjuan Xi
A photocatalytic CO2-promoted divergent C(sp3)–H carboxylation of benzyl alcohols was developed. This redox-neutral process achieves superior atom economy, transforming simple feedstocks into value-added functionalized acids.
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Enantiocomplementary synthesis of chiral 2,3-dihydroxy aryl ketones via ThDP-dependent enzymatic catalysis
DOI: 10.1039/D6GC01483F, PaperDan Li, Zheng Zhu, Xiaoyu Chen, Xuesi Chen, Liming Ouyang, Huangong Li, Lixin Zhang, Yongtao Xie
A green and enantiocomplementary biocatalytic platform for chiral 2,3-dihydroxy aryl ketones has been developed.
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Machine learning to predict plasma-based CO2 conversion in dielectric barrier discharge reactors
DOI: 10.1039/D6GC01077F, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Jiayin Li, Xinpei Lu, Pranav Arun, Jing Xu, Fausto Gallucci, Sirui Li, Annemie BogaertsA hybrid ML model trained on 358 cross-study data points predicts CO2 conversion in DBD reactors with an R2 of 0.92 on unseen experiments, providing an unbiased assessment of model generalizability across heterogeneous experimental sources.
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Efficient methanolysis of PET to produce high-purity DMT via homo-heterogeneous Mn2+/Mn2O3 synergistic catalysis
DOI: 10.1039/D6GC01939K, PaperLei Yang, Jiacheng Gao, Min Su, Li Yuan, Yuan Wang, Dajun Wang, Heng Zheng, Shaojun Yuan, Like Ouyang
This study develops a synergistic MnCl2·4H2O/Mn2O3 system which enables efficient PET methanolysis to produce high-purity DMT (95.35% yield) via a dynamic Mn2+/Mn3+ interface, with Aspen simulation confirming its economic viability.
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Multi-physical field synergistic driving for solar-driven interfacial evaporation: mechanisms, strategies and system optimization
DOI: 10.1039/D6GC01760F, Critical ReviewChongjia Fang, Haixin Guo, Xinhua Qi
This review analyzes solar-driven interfacial water evaporation from a multi-physical field coupling perspective, focusing on the trade-off between evaporation flux and salt resistance.
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Research progress on the synergistic promotion of the water splitting process by oxyanions
DOI: 10.1039/D6GC00582A, Tutorial ReviewWenwen Zi, Jinhua Huang, Xinyue Zhang, Meng Zhang, Junjun Zhang
This review summarizes the research progress on the synergistic promotion of the water splitting process by oxyanions.
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Integrating mechanochemical synthesis of a pyridinium-based graphitic ionic framework into an eco-friendly gold recycling process
DOI: 10.1039/D5GC06936J, PaperZhi-Wei Liu, Zhizhuo Yang, Zhaoying Zhang, Xilin Gao, Chuanying Liu, Chengliang Xiao
This work combines mechanochemical GIF-4 synthesis with benign leaching for green gold recovery, enabling excellent Au(III) capture from e-waste with a reduced ecological footprint.
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Photothermal catalytic CO2 oxidative dehydrogenation of propane over an oxygen-vacancy-rich perovskite-type CeNiO3 catalyst
DOI: 10.1039/D6GC01194B, PaperChun-Fei Li, Zhen-Hong He, Mei-Xia Yang, Yu-Xuan Ji, Sen-Wang Wang, Meng-Nan Liu, Weitao Wang, Kuan Wang, Huan Wang, Zhao-Tie Liu
A perovskite-type CeNiO3 catalyst rich in oxygen vacancies can efficiently achieve photothermal catalytic CO2 oxidative dehydrogenation of propane.
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Photocatalytic hydrogenolysis of C–O bonds in lignin model compounds and lignin bio-oil over Ru-supported holey g-C3N4 exfoliated nanosheets
DOI: 10.1039/D5GC06461A, PaperHimanshu Dhiman, Arjun K. Manal, Rajendra Srivastava
Thermally exfoliated Ru/ECNHS enabled efficient photocatalytic valorization of α-O-4, β-O-4, and 4-O-5 C–O linkages in lignin-derived aryl ethers and native lignin into value-added hydrocarbons and oxygenates.
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Highly efficient microwave-accelerated transfer hydrogenation for CO2-derived carbonate valorization by Ru(II)–protic-NHC pincer catalysts
DOI: 10.1039/D6GC00476H, PaperAchena Saha, Shambhu Nath, Ekta Yadav, Amrendra K. Singh
Ru–pNHC catalysts show record activity in the microwave-accelerated transfer hydrogenation of inorganic carbonates with glycerol to form lactate (TOF 5.8 × 105 h−1) and formate (TOF 1.6 × 105 h−1), advancing CO2 valorization and hydrogen storage.
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