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Fully-biobased Monomers Containing Monopyrrolidone Ring Towards the Synthesis of Renewable Polyesters with High Tg and Hydrolyzable Closed-loop Recycling
Green Chem., 2026, Accepted Manuscript
DOI: 10.1039/D5GC05862G, PaperYumeng Zhang, Yang Yu, Ziyi Feng
The development of fully bio-based polyesters with distinguished performance and facile chemical closed-loop recycling in aqueous environment still faces a challenge. Herein, a series of N-substituted pyrrolidone carboxylic acid monomers...
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DOI: 10.1039/D5GC05862G, PaperYumeng Zhang, Yang Yu, Ziyi Feng
The development of fully bio-based polyesters with distinguished performance and facile chemical closed-loop recycling in aqueous environment still faces a challenge. Herein, a series of N-substituted pyrrolidone carboxylic acid monomers...
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Establishing Parameters for Resonant Acoustic Mixing (RAM) Chemistry using Buchwald-Hartwig Amination as a Model
Green Chem., 2026, Accepted Manuscript
DOI: 10.1039/D6GC00784H, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Lori Gonnet, Cameron B. Lennox, Tristan H Borchers, Mohammad Askari, Alexander Wahrhaftig-Lewis, Stefan G Koenig, Karthik Nagapudi, Tomislav Friščić
While Resonant Acoustic Mixing (RAM) has been proposed as a scalable methodology for environmentally-friendly synthesis, notably media-free mechanochemical synthesis, the underlying reaction environment and the parameters that govern reaction control,...
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DOI: 10.1039/D6GC00784H, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Lori Gonnet, Cameron B. Lennox, Tristan H Borchers, Mohammad Askari, Alexander Wahrhaftig-Lewis, Stefan G Koenig, Karthik Nagapudi, Tomislav FriščićWhile Resonant Acoustic Mixing (RAM) has been proposed as a scalable methodology for environmentally-friendly synthesis, notably media-free mechanochemical synthesis, the underlying reaction environment and the parameters that govern reaction control,...
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Highly enantioselective epoxidation of trisubstituted vinyl sulfones with H2O2 catalyzed by a bioinspired manganese catalyst
DOI: 10.1039/D5GC06431G, PaperWanting Tong, Yirui Chen, Xinhang Jin, Hangtao Wu, Chaoran Xu, Dingguo Song, Fei Ling, Weihui Zhong
Highly enantioselective epoxidation of trisubstituted alkenyl sulfones is achieved using a Mn catalyst with a p-methoxybenzyl arm that remotely tunes steric and electronic effects to enhance stereocontrol.
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Metal-free carbocatalysts for the selective production of ethylbenzene and cumene from mixed plastic waste
Green Chem., 2026, Accepted Manuscript
DOI: 10.1039/D5GC06756A, PaperWahyu Dewi, Jinxing Gu, Fatima Shahid, Nauman Ahmad, I. M. S. K. Ilankoon, Alan L Chaffee, Lian Zhang
Conventional production of ethylbenzene and cumene relies on fossil fuels and results in significant CO2 emissions. As a sustainable alternative, plastic waste can be used to produce high-value aromatics via...
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DOI: 10.1039/D5GC06756A, PaperWahyu Dewi, Jinxing Gu, Fatima Shahid, Nauman Ahmad, I. M. S. K. Ilankoon, Alan L Chaffee, Lian Zhang
Conventional production of ethylbenzene and cumene relies on fossil fuels and results in significant CO2 emissions. As a sustainable alternative, plastic waste can be used to produce high-value aromatics via...
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Replacing low-boiling-point amines: electrocatalytic phosphinamide synthesis with liquid formamide reagents
DOI: 10.1039/D5GC06344B, PaperHang Gong, Jingao Xiao, Hui Gao, Kexiao Zhou, Rong Yang, Changqun Cai
This work presents an electrocatalytic strategy for safe and efficient phosphinamide synthesis using liquid formamides, avoiding volatile low-boiling amines. This metal- and oxidant-free method offers a versatile platform for green synthesis.
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Muconic acid: a renewable platform monomer for polymer materials
DOI: 10.1039/D6GC00103C, Tutorial ReviewAocheng Wei, Qinyang Lei, Xiaomeng You, Xiaojun Shen, Lin Dai, Tong-Qi Yuan
Muconic acid occupies a pivotal position at the confluence of biology, chemistry, and industrial technology. Synthesis and polymerization of muconic acid hold promise advanced materials and applications.
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Turning light into carbinols: a metal-free radical strategy for pyridine based triaryl scaffolds
DOI: 10.1039/D5GC05657H, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Matteo Leone, Maurizio FagnoniWe propose a photoinduced synthesis of Triaryl Carbinols, achieved under mild and metal-free conditions via radical addition of benzophenones to cyanopyridines.
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Lessons learned on how to reengineer enzymes for improved performance in ionic liquids: insights from BSLA saturation mutagenesis library
DOI: 10.1039/D5GC04809E, Critical Review
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Shuaiqi Meng, Yu Ji, Maxine Yew, Leilei Zhu, Ulrich SchwanebergBased on a complete BSLA saturation mutagenesis library, this review shows how ionic liquids reshape enzyme solvation and performance. Preserving and modulating the hydration shell emerges as a key design principle for IL-tolerant biocatalysts.
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Lignocellulosic biomass in electrochemical energy conversion and value-added chemicals production
DOI: 10.1039/D5GC06399J, Critical ReviewGuohao Xu, Xiaotong Chen, Weizhuo Xu, Qiujin Shi, Yun Lu, Wei Liu
This review highlights the electrochemical conversion of lignocellulosic biomass into clean energy and value-added chemicals, with a specific focus on key future directions.
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Chemical affinity guided high-valence metal oxide interphase engineering for upcycling of ternary cathodes from electric vehicles
DOI: 10.1039/D5GC07089A, PaperWenyu Wang, Renming Zhan, Yuanjian Li, TianCheng Dong, Zihe Chen, Ruikang Feng, Yida Lu, Yongming Sun
Chemical affinity guided interphase engineering upcycles electric-vehicle cathodes materials for durable high-voltage and high-temperature cycling, enabling sustainable lithium-ion battery recycling.
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Cascading integration of genetic-reduced cellulose nanofibers and ultrasound-dissected fungi mycelium for synergistic enhancements of cellulases and saccharification with high-performance bioproducts
Green Chem., 2026, Accepted Manuscript
DOI: 10.1039/D5GC06304C, PaperHao Peng, Peng Liu, Jingyuan Liu, Junsheng Yu, Boyang He, Yujing Yang, Hua Yu, Heng Kang, Mengzhou Zhou, Wanbin Zhu, Muhammad Nauman Aftab, Yanting Wang, Chunxang Fu, Liangcai Peng
Plants provide enormous biomass resources convertible for biofuels and bioproducts, but lignocellulose recalcitrance signifies a critical difficulty to achieve the optimal enzymes complexes that are universally capable for diverse biomass...
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DOI: 10.1039/D5GC06304C, PaperHao Peng, Peng Liu, Jingyuan Liu, Junsheng Yu, Boyang He, Yujing Yang, Hua Yu, Heng Kang, Mengzhou Zhou, Wanbin Zhu, Muhammad Nauman Aftab, Yanting Wang, Chunxang Fu, Liangcai Peng
Plants provide enormous biomass resources convertible for biofuels and bioproducts, but lignocellulose recalcitrance signifies a critical difficulty to achieve the optimal enzymes complexes that are universally capable for diverse biomass...
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Synergistic nickel phthalocyanine integration on carbon nitride for improved selective nitrogen reduction to ammonia
DOI: 10.1039/D5GC06417A, PaperSourav Bhowmick, Narad Barman, Amal Gain, Ashadul Adalder, Rajashri Urkude, Biplab Ghosh, Sourav Mukherjee, Supriya Mondal, Ranjit Thapa, Uttam Kumar Ghorai
As a sustainable alternative to the energy-intensive Haber–Bosch process, the electrochemical nitrogen reduction reaction (eNRR) offers a promising green approach for converting abundant atmospheric nitrogen into ammonia.
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Electrocatalytic oxidation or amidation of olefins by asymmetric electrolytes steering carbocation pathways
DOI: 10.1039/D5GC07050C, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Yingxuan Zhao, Chenyang Shen, Qing Liu, Siyuan Zhao, Ruiyao Zhao, Xiangke Guo, Nianhua Xue, Luming Peng, Xuefeng Guo, Yan Zhu, Weiping DingAsymmetric electrolytes precisely control olefin-derived carbocations, enabling complete oxidation (ECOR) or Ritter amidation (ECAR, 98%) with >65% faradaic efficiency, providing a sustainable route to obtain valuable N- and O-containing compounds.
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Tunable electrochemical oxidation of bisphosphines: a general strategy for selective synthesis of bidentate phosphine mono- and dioxides
DOI: 10.1039/D5GC06594A, PaperRong Yang, Jingao Xiao, Xiujuan Zhang, Rui Yang, Changqun Cai, Hang Gong
Tunable electrochemical oxidation of bisphosphines enables selective synthesis of bidentate phosphine monooxides (BPMOs) and dioxides (BPDOs) by adjusting current, a metal-and-oxidant-free method using DMF as oxygen source for ligand synthesis.
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CarAT: carbon atom tracing across industrial chemical value chains via chemistry language models
DOI: 10.1039/D5GC04348D, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Emma Pajak, David Walz, Olga Walz, Laura Marie Helleckes, Klaus Hellgardt, Antonio del Rio ChanonaCarAT is a molecular-level framework for tracing carbon through industrial value chains, enabling biogenic carbon accounting to support crade-to-grave assessments, inform decarbon.
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Production of furanics from sugarcane bagasse via the 5-chloromethylfurfural pathway: techno-economics and greenhouse gas assessment
DOI: 10.1039/D5GC05170C, PaperJerome Ramirez, Aban Sakheta, Lalehvash Moghaddam, Darryn Rackemann, Gabriel Fraga
This study investigated the commercial-scale production of furan-based chemicals (furanics) from sugarcane bagasse, using 5-chloromethylfurfural (CMF) as an intermediate platform molecule for the production of bio-based chemicals and materials.
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Solvent-controlled divergent 1,2-dialkylation and 1,1,2-bromodialkylation of terminal alkynes to access difluoroalkylated cyclopentanes
DOI: 10.1039/D5GC06365E, CommunicationJianguo Han, Yatao Lang, Chen Zhu, Huifeng Yue
We have developed a mild and efficient photocatalytic strategy that enables both 1,2-difunctionalization and 1,1,2-trifunctionalization of terminal alkynes with bromodifluoroacetates, simply by switching the reaction solvent.
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Interfacial electronic engineering of co-doped Ni(OH)2 nanoarrays for efficient electrooxidation of xylose to formate
DOI: 10.1039/D6GC00334F, PaperJianyun Gan, Ning Wang, Yunpeng Liu, Zhendong Liu, Bo Lu, Yongfa Huang, Ge Yuan, Emmanuel Iwuoha, Ruidong Xia, Ren Zou, Xinwen Peng
Ni–O–Co covalent bridges from Co doping function as electron relay pathways, facilitating rapid pre-oxidation and continuous charge transfer to enable a fast Ni3+/Ni2+ redox cycle for efficient low-potential xylose oxidation to formate.
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Controlling the free volume of type III porous liquids by tailoring solvent for enhanced CO2 capture
DOI: 10.1039/D5GC06493G, PaperPingping Zhao, Zhihao Li, Baikang Dong, Xin Su, XuanXuan Li, Fengling Wang, Qiang Wang, Di Liu, Dongmei Xu, Jun Gao
DBU-based porous liquids (PLs) were employed for the improvement of CO2 absorption capacity via a unique internal driving force from the synergistic effect between the absorption active sites and the nano-confined spaces of the interface of PLs.
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Unveiling the triple enhancement mechanism of phosphorus doping: a carbon cathode with a precise mesoporous structure for advanced zinc-ion energy storage
DOI: 10.1039/D5GC06750B, PaperYongtao Sun, Ying Li, Huihui Li, Shengqin Guan, Jianlong Wang, Binbin Zhang, Shengliang Hu, Kaixi Li, Taotao Guan
Structural instability of high-surface-area, large-pore-volume carbons during electrochemical cycling is addressed by a dual-function strategy of precise pore regulation via self-assembly and in-situ heteroatom anchoring.
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